Abstract

We present experimental results on the characteristic sharing of available excess energy, ranging from 11–221 eV, between two electrons in single-photon direct double ionization of He. An effective parametrization of the sharing distributions is presented along with an empirical model that describes the complete shape of the distribution based on a single experimentally determinable parameter. The measured total energy sharing distributions are separated into two distributions representing the shake-off and knock-out parts by simulating the sharing distribution curves expected from a pure wave collapse after a sudden removal of the primary electron. In this way, empirical knock-out distributions are extracted and both the shake-off and knock-out distributions are parametrized. These results suggest a simple method that can be applied to other atomic and molecular systems to experimentally study important aspects of the direct double ionization process.

Highlights

  • We present experimental results on the characteristic sharing of available excess energy, ranging from 11–221 eV, between two electrons in single-photon direct double ionization of He

  • If the photon energy is higher than the double ionization potential, there will be a probability for the secondary electron to be ‘shaken off ’ by a wave collapse into states with both electrons in the continuum

  • SO from the ground state in He would be characterized by the primary electron going out as a p-wave, as it takes the angular momentum of the absorbed photon, and the secondary electron as an s-wave

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Summary

Introduction

We present experimental results on the characteristic sharing of available excess energy, ranging from 11–221 eV, between two electrons in single-photon direct double ionization of He. The primary electron, i.e. the one that interacts with the photon, transfers some of its energy to the secondary electron by a collision-like process. Such a process can lead to double ionization when the energy is shared in such way that both electrons receive a sufficient amount of additional kinetic energy that they can leave the system. This collision-like mechanism is called the knock-out (KO) mechanism.

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