Abstract
We investigate solid hydrogen as a nonlinear optical medium. We carry out stimulated Raman scattering (SRS) experiments using a large Raman coherence prepared with two single frequency pulsed lasers. We show that multiorder SRS generation proceeds collinearly to the pump beam axis without stringent restriction of phase matching. We show also that the SRS generation dominantly occurs for negative two-photon detunings for which the Raman coherence can follow the antiphased state coherence.
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