Parallel measurement of conductive and convective thermal transport of micro/nanowires based on Raman mapping

Abstract

Heat conduction and convection are coupled effects in thermal transport of low-dimensional materials especially at micro/nanoscale. However, the parallel measurement is a challenge due to the limitation of characterization pathways. In this work, we report a method to study conductive and convective thermal transport of micro/nanowires simultaneously by using steady-state Joule-heating and Raman mapping. To examine this method, the carbon nanotubes (CNTs) fiber (36 μm in diameter) is characterized and its temperature dependence of thermal properties including thermal conductivity and convection coefficient in ambient air is studied. Preliminary results show that thermal conductivity of the CNTs fiber increases from 26 W/m K to 34 W/m K and convection coefficient decreases from 1143 W/m2 K to 1039 W/m2 K with temperature ranging from 312 to 444 K. The convective heat dissipation to the air could be as high as 60% of the total Joule heating power. Uncertainty analysis is performed to reveal that fitting errors can be further reduced by increasing sampling points along the fiber. This method features a fast/convenient way for parallel measurement of both heat conduction and convection of micro/nanowires which is beneficial to comprehensively understanding the coupled effect of micro/nanoscale heat conduction and convection.