Abstract
Palladium(0) nanoparticles supported on the external surface of Cu3(btc)2 framework (PdNPs@Cu3(btc)2) were in-situ generated from the reduction of Pd(acac)2 precursor impregnated on the Cu3(btc)2 support during the dehydrogenation of dimethylamine-borane in toluene at room temperature. The characterization of PdNPs@Cu3(btc)2 by using advanced analytical techniques shows the formation of well-dispersed palladium(0) nanoparticles supported on Cu3(btc)2 surface. These new palladium(0) nanoparticles were found to be the most active and the longest-lived nanocatalyst with superior reusability performance in the dehydrogenation of dimethylamine-borane at room temperature.
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