Abstract
A task-specific ionic liquid strategy was, for the first time, proposed for designing oxygen vacancy-rich α-Fe2O3 nanocubes toward electrocatalytic N2 fixation to NH3 under ambient conditions, offering a NH3 formation rate of 32.13 μg h-1 mgcat-1 with a faradaic efficiency of 6.63% at -0.3 V vs. the reversible hydrogen electrode.
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