Abstract
Kinetic isotope effects (KIEs) during the oxidative coupling of methane over a Li + /MgO catalyst at 700 o C have been determined using several different experimental methods and by a reaction model that includes both heterogeneous and homogeneous reactions. By maintaining a constant partial pressure of methane of 190 Torr and changing the partial pressure of oxygen, a variation in the H/D KIE, based on differing rates of CH 4 and CD 4 conversion, was observed
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