Abstract
Double resonance optically pumped magnetometry can be used to measure static magnetic fields with high sensitivity by detecting a resonant atomic spin response to a small oscillating field perturbation. Determination of the resonant frequency yields a scalar measurement of static field ($B_0$) magnitude. We present calculations and experimental data showing that the on-resonance polarimeter signal of light transmitted through an atomic vapour in arbitrarily oriented $B_0$ may be modelled by considering the evolution of alignment terms in atomic polarisation. We observe that the amplitude and phase of the magnetometer signal are highly dependent upon $B_0$ orientation, and present precise measurements of the distribution of these parameters over the full 4{\pi} solid angle.
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