Abstract
Abstract Stereoselective syntheses of N,N-bis(dihydrofuranyl)hydroxyamines from phenols and nitroolefins have been accomplished by means of cycle-specific catalysis with guanidine/bisthiourea organocatalyst and achiral base. Circumstantial evidence supports the idea that a nitroso intermediate participates in the dimerization, which involves internal redox reaction/umpolung.
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