Abstract

The paper reports synthesis and co-crystallization of 5 co-crystal of 4-nitrophenol (4N) with five different monoand diaminopyridines (4-aminopyridine (4AP); 3,4-diaminopyridine (34DAP); 2-amino-6-methylpyridine (26MAP); 2,6- diaminopyridine (26DAP); 2-aminopyridine (2AP)) resulted in five adducts with the molar ratio of components 2:1 in final compounds. X-ray analysis confirms the non-centrosymmetric packing of obtained compounds. Two compounds crystallize in the polar acentric P2<sub>1</sub> and three compounds crystallize in acentric orthorhombic Pna2<sub>1</sub> space groups. The comparative studies on the laser induced multiple and single shot damage thresholds of named crystals were carried out using radiation of 1064 nm from Nd:YAG laser with pulse width 10 ns. Obtained results show good laser-induced singleshot and multiple-shot damage threshold values for all studied co-crystals and are found up to 3.64 GW/cm<sup>2</sup> and 1.77 GW/cm<sup>2</sup> respectively.

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