Abstract

• Fully solution-derived GQDs-IGZO TFTs based on ZrO 2 as gate dielectrics have been achieved. • GQDs-IGZO TFTs devices with optimized doping content have demonstrated improved performances, including a μ FE of 35.91 cm 2 V –1 s –1 , a higher I ON / I OFF of 5.04 × 10 8 , a smaller subthreshold swing (SS) of 0.11 V dec –1 and a smaller interfacial trap states of 1.57 × 10 12 cm −2 . • Resistor-loaded unipolar inverter based on GQDs-IGZO/ZrO x has been integrated, demonstrating good dynamic behavior and a high gain of 9.3. • LFN characteristics of GQDs-IGZO/ZrO x TFTs have suggested that the fluctuations in mobility are the noise source. This work presents solution-processed high-performance graphene quantum dots (GQDs) decorated amorphous InGaZnO (α-IGZO) thin-film transistors (TFTs) based on ZrO x as gate dielectrics. Compare with pure IGZO TFTs, GQDs-modified α-IGZO TFTs devices with optimized doping content have demonstrated better performances, including a larger field-effect mobility ( μ FE ) of 35.91 cm 2 V –1 s –1 , a higher on/off current ratio ( I ON / I OFF ) of 5.04 × 10 8 , a smaller subthreshold swing (SS) of 0.11 V dec –1 and a smaller interfacial trap states ( D it , 1.57 × 10 12 cm −2 ). Moreover, the GQDs-doped IGZO TFTs with a doping concentration of 0.5 mg ml –1 have shown excellent stability under bias stress and illumination stress conditions. To demonstrate the potential applications of α-IGZO TFTs in logic circuits, a resistor-loaded unipolar inverter based on GQDs-IGZO/ZrO x has been integrated, demonstrating good dynamic behavior and a high gain of 9.3. Low-frequency noise (LFN) characteristics of GQDs-IGZO/ZrO x TFTs have suggested that the fluctuations in mobility are the noise source. Based on all the experimental findings, it can be concluded that solution-processed GQDs-IGZO/ZrO x TFT may envision promising applications in optoelectronics.

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