Abstract
A computer-automated design process for a surface-enhanced Raman scattering (SERS) substrate using a particle swarm optimization algorithm is proposed. Nanostructured Ag coated hydrogen silsesquioxane nanopillar arrays of various sizes for SERS substrate applications are fabricated by direct Ag film deposition on substrates patterned by electron beam lithography and are investigated systematically. Good agreement is demonstrated between experimental and simulation results. The absorption spectra, charge distributions, and electric field distributions are calculated using finite-difference time-domain simulations to explain the field enhancement mechanism and indicate that this enhancement originates from plasmon resonance. Our work provides a guide towards optimum SERS substrate design.
Published Version
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