On the photomultiplier-tube asymmetry in liquid scintillation counters for the CIEMAT/NIST efficiency tracing method

Abstract

The triple-to-double coincidence ratio (TDCR) and the CIEMAT/NIST efficiency tracing (CNET) methods are important techniques for accurate activity determination in radionuclide metrology and other fields. The methods require liquid scintillation (LS) counters with three (TDCR) or two (CNET) photomultiplier tubes (PMTs), respectively, and the original techniques assume that the responses of all PMTs in a counter system are identical. This assumption is, however, often not fulfilled. This may have significant consequences for the activity determination, and dedicated corrections are required. Corresponding effects and possible corrections for the TDCR method were discussed in a recent article (Kossert et al., 2020) while the CNET method was not included in that work. The intention of this paper is to present a brief theoretical consideration of this problem. This paper makes clear that for most radionuclides potential PMT asymmetries in CNET counters are of minor importance. In addition, measures to identify potential asymmetries in these counters are discussed.