Abstract
We investigate the origin and nature of femtosecond time-resolved (TR) pump–probe differential (PPD) signal from the exciton resonance in semiconductor quantum wells (QWs) in the coherent regime. The excitonic PPD signal is expressed as a sum of interferences of the excitonic nonlinear polarization with the incident probe field and the linear polarization induced by the probe. A nonzero excitonic TR-PPD signal from QWs can occur for time t larger than the pulse width ( t p) when the exciton dephasing time is longer than t p, and this signal can originate only from the second interference term for both the negative and positive pump–probe delays, the contribution from the first interference term being zero for t> t p. This is in contrast with the case of PPD signal in the spectral domain where the first interference term plays a major role. We discuss the effects of many body interactions on the TR-PPD signal. It is shown that excitation-induced dephasing can cause a significant increase in the rise time of the TR-PPD signal.
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