Abstract
The Green's function approach is used for the calculation of double ionization energies of methane and silane. The results obtained for methane compare quantitatively with the experimental Auger data and with those previously obtained by configuration interaction calculations. The double ionization energies obtained for the silane molecule also give a quantitative account of the gas-phase L 2,3MM Auger spectrum and allow for its unambiguous assignment. This assignment differs from the one originally proposed on qualitative grounds.
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