On/off switchable interfacial thermal resistance in graphene/fullerene/graphene heterostructures

Abstract

Switchable thermal devices are attracting significant research interest as a basic thermal management component. In this work, taking graphene/fullerene/graphene sandwiches as an example, we demonstrate that the interfacial thermal resistance can show a switchable, step-like change by varying the number of fullerenes in the sandwich structure. Changing the number of fullerenes causes a structural transition between the graphene layers from adhered to separated, resulting in an enhancement of about a factor of two in the interfacial thermal resistance during this on/off switchable phenomenon, which we analyze using analytic expressions based on the thermal transport theory. We further illustrate that the switchable phenomenon can also be realized by applying mechanical strain or by varying the temperature of the sandwich structure. This work demonstrates that the sandwich-liked nanoscale heterostructures can exhibit hysteretic changes in heat transport, and thus have promise for potential applications in switchable thermal devices.