Abstract
Photo‐induced effects have been detected by magnetic measurements, Mossbauer spectroscopy and reflectivity. The LIESST effect has been achieved in the spin‐crossover system [FexCo1-x(btr)2(NCS)2]·H2O. We investigated the purely photo‐induced magnetism of a Prussian Blue analogue Rb0.52Co[Fe(CN)6]0.84, 2.31 H2O, involving an optical electron transfer from FeII to CoIII. Inherent aspects of photomagnetic experiments are described: bulk and surface effects, magnetic and electronic metastabilities of the photo‐excited state.
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