Abstract
Olefin radical cations are characterized by time-resolved fluorescence-detected magnetic resonance (FDMR) in pulse radiolysis of saturated hydrocarbons. Studies of both neat and mixed saturated hydrocarbon fluids by FDMR at low temperature(to≈ 100°C) suggest that olefin cations originate in the fragmentation of (vibrationally) excited (parent) saturated hydrocarboncations.
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