Abstract
Sewage treatment plants effectively remove silver (Ag) from sewage. Sewage sludge can therefore be important Ag sinks, polluting the environment with this element. In this work, we report a nation-wide survey on the Ag content of sewage sludge in China (0.23-19.02 mg kg-1, average 2.72 mg kg-1). Furthermore, we identify that sludge disposal represents an important Ag pollution source (84.48 tons in 2016) for the environment by estimating the national and provincial inventories of sludge-borne Ag in China. Also the positive correlations between the per capita gross domestic product (GDP)/provincial GDP and the content/mass loadings of Ag highlighted the impact of human activities on Ag pollution. In different samples, strong complexation of thiosulfate contributed to the highest leaching concentration (95.00-438.15 μg kg-1) and ratio (1.9-8.8%) of Ag, emphasizing the necessity of a long-term risk assessment for landfill and land application of sludge.
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