Abstract

We present electron and nuclear dynamic imaging of a polyatomic molecule in an ultrashort intense laser pulse. A numerical solution of the time-dependent Schrödinger equation is described to study the non-perturbative nonlinear dynamic of a nonlinear polyatomic molecule in interaction with ultrashort intense laser pulse. In a quantum description of the molecular system, beyond the Born-Oppenheimer approximation, we investigate the full influence of the nuclear motion on the photoionization and harmonic generation processes.

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