Abstract

Collinear laser spectroscopy measurements were performed on $^{69,71,73}$Ge isotopes ($Z = 32$) at ISOLDE-CERN. The hyperfine structure of the $4s^2 4p^2 \, ^3P_1 \rightarrow 4s^2 4p 5s \, ^3P_1^o$ transition of the germanium atom was probed with laser light of 269 nm, produced by combining the frequency-mixing and frequency-doubling techniques. The hyperfine fields for both atomic levels were calculated using state-of-the-art atomic relativistic Fock-space coupled-cluster calculations. A new $^{73}$Ge quadrupole moment was determined from these calculations and previously measured precision hyperfine parameters, yielding $Q_{\rm s}$ = $-$0.198(4) b, in excellent agreement with the literature value from molecular calculations. The moments of $^{69}$Ge have been revised: $\mu$ = +0.920(5) $\mu_{N}$ and $Q_{\rm s}$= +0.114(8) b, and those of $^{71}$Ge have been confirmed. The experimental moments around $N = 40$ are interpreted with large-scale shell-model calculations using the JUN45 interaction, revealing rather mixed wave function configurations, although their $g$-factors are lying close to the effective single-particle values. Through a comparison with neighboring isotones, the structural change from the single-particle nature of nickel to deformation in germanium is further investigated around $N = 40$.

Highlights

  • Over the years, structural changes have been intensively investigated in the region between the semimagic 68Ni and the doubly magic 78Ni [1,2,3,4,5,6]

  • The germanium ions were accelerated to 50 keV, mass separated using the high-resolution isotope separator (HRS) and subsequently cooled and bunched in a gas-filled linear Paul trap (ISCOOL) [26]

  • The systematic analysis of the hfs of 69,71,73Ge isotopes obtained in this work requires a revision of the hyperfine constants for 69Ge, resulting in different magnetic and quadrupole moments

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Summary

Introduction

Structural changes have been intensively investigated in the region between the semimagic 68Ni and the doubly magic 78Ni [1,2,3,4,5,6]. The nuclear properties of ground and isomeric states, such as spins, moments, and charge radii, have made significant contributions in elucidating the above-mentioned nuclear phenomena. This was achieved by laser spectroscopy measurements on the isotopic chains of nickel (Z = 28), copper (Z = 29), zinc (Z = 30), and gallium (Z = 31) [3,5,6,7,8,11,13,14,15,16,17,18]. Nuclear spins and magnetic dipole moments are sensitive probes of the single-particle nature or configuration mixing of the wave functions [5,6,8,11], while the electric quadrupole moment and charge radii tell us more about the nuclear shape and collectivity [3,13,14]

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