Abstract
Nowadays, radon gas exposure is considered one of the main health concerns for the population because, by carrying about half the total dose due to environmental radioactivity, it is the second cause of lung cancer after smoking. Due to a relatively long half-life of 3.82 days, the chemical inertia and since its parent Ra-226 is largely diffuse on the earth’s crust and especially in the building materials, radon can diffuse and potentially saturate human habitats, with a concentration that can suddenly change during the 24 h day depending on temperature, pressure, and relative humidity. For such reasons, ‘real-time’ measurements performed by an active detector, possibly of small dimensions and a handy configuration, can play an important role in evaluating the risk and taking the appropriate countermeasures to mitigate it. In this work, a novel algorithm for pattern recognition was developed to exploit the potentialities of silicon active detectors with a pixel matrix structure to measure radon through the α emission, in a simple measurement configuration, where the device is placed directly in air with no holder, no collection filter or electrostatic field to drift the radon progenies towards the detector active area. This particular measurement configuration (dubbed as bare) requires an α/β-discrimination method that is not based on spectroscopic analysis: as the gas surrounds the detector the α particles are emitted at different distances from it, so they lose variable energy amount in air depending on the traveled path-length which implies a variable deposited energy in the active area. The pixels matrix structure allows overcoming this issue because the interaction of α, β and γ particles generate in the active area of the detector clusters (group of pixels where a signal is read) of different shape and energy dispersion. The novel algorithm that exploits such a phenomenon was developed using a pixelated silicon detector of the TimePix family with a compact design. An α (Am-241) and a β (Sr-90) source were used to calibrate the algorithm and to evaluate its performances in terms of β rejection capability and α recognition efficiency. Successively, the detector was exposed to different radon concentrations at the ENEA-INMRI radon facility in ‘bare’ configuration, in order to check the linearity of the device response over a radon concentration range. The results for this technique are presented and discussed, highlighting the potential applications especially the possibility to exploit small and handy detectors to perform radon active measurements in the simplest configuration.
Highlights
Radon (Rn-222) is a naturally occurring radioactive gas produced by the decay of theRa-226 radionuclide which is largely diffused on the earth’s crust as well as in building materials, as it belongs to the natural U-238 chain
The main techniques used to monitor radon activity concentration in air are two: (i) integration techniques, generally used by passive detectors like dosimeters or electrets [7,8,9,10], which return the integral value of radon concentration measured over the time period of the detector exposure and (ii) real-time techniques, performed by active detectors, that perform radon concentration measurements on small pre-set time intervals, that can be repeated over the total time of exposure
The results presented in this work show the feasibility of exploiting a pixelated silicon detector to measure the radon concentration through its α emitting progeny in ‘bare’ configuration, thanks to the application of the novel algorithm developed
Summary
Radon (Rn-222) is a naturally occurring radioactive gas produced by the decay of theRa-226 radionuclide which is largely diffused on the earth’s crust as well as in building materials, as it belongs to the natural U-238 chain. The inhalation of radon, and in particular of its α emitters daughters like Po-218 and Po-214, is one of the main causes of lung cancer due to the high ionizing power of the emitted α particles which can damage cells and DNA inside the nucleus [1,2,3,4]. For these reasons, the World Health Organization (WHO) considers radon gas as one of the main health concerns among those related to environmental radioactivity exposure [5,6], carrying almost half the total dose due to environmental radiation. Real-time measurements of radon concentration in air assume a fundamental importance to monitor the exposure variation over the proper timescale, allowing to promptly undertake the appropriate countermeasures to mitigate the risk
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