Abstract

Experiments reveal a new family of optical fields that originate at the boundary between a nanostructure and an incident light source, offering new paths for controlling optical behavior in a wide range of technologies.

Highlights

  • Physical interactions typically occur within a structure, designed to concentrate the continuous distribution of system states around discrete eigenstates

  • We propose and implement the concept of nonmodal plasmonics, rooted in the fact that light sources and nanostructures actively share a principal set of discrete optical degrees of freedom

  • We discover a new class of plasmonic DOFs, identified not with the modes of photonic nanostructures but with the discrete antiresonances that form when those nanostructures are being driven by a light source

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Summary

INTRODUCTION

Physical interactions typically occur within a structure, designed to concentrate the continuous distribution of system states around discrete eigenstates. These discrete eigenstates constitute the principal degrees of freedom (DOFs) controlling the predominant mechanisms of interaction. Whereas SPPs are discrete resonances of free plasmonic oscillations, APPs are the discrete antiresonances emerging when those oscillations are being forced by a light source [Figs. These SPP-APP pair excitations, we demonstrate that ultrathin gold films (approximately 11 nm) can appear “black”: exhibiting a surprisingly strong angularly and spectrally wideband absorption (FWHM Δθ ≈ 47°, Δλ > 1.34 μm). We derive design rules to engineer highly absorbing ultrathin films accurately and efficiently based on the unique properties of SPP-APP pairs

THEORY
EXPERIMENT
WIDEBAND ABSORPTION BY ULTRATHIN GOLD FILMS
DISCUSSION AND SUMMARY
Mapping the backscattering process to a scalar linear system
Linear independence of the discrete resonant and antiresonant field solutions
Experimental setup
Sample preparation
Sample characterization
Calculating the long-range SPP and APP dispersion relations
Calculating the predicted reflectance signature
SPP-APP pair trajectory in momentum-energy space
The excitation direction dependence of APPs
Mutual deflection in the line shape of an SPP-APP pair
Designing for the black gold film effect
Approximating the angular reflectance with a Fano model
Failure of the Fano model for ultrathin films
Findings
Intrinsic limitations of the Fano model

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