Abstract
Abstract The third principle of group theoretical statistical mechanics is used to define the existence of many new nonlinear optical rotatory phenomena caused by the interaction of intense electromagnetic radiation with molecular ensembles. This treatment removes the necessity of having to distinguish between ‘natural’ and ‘magnetic’ optical activity; both processes emerge consistently from the analysis, which is based on an application of the Hellman-Feynman theorem and a double Taylor expansion of the induced electric and magnetic dipole moments.
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