Abstract

Chiral anomaly is a distinct quantum anomaly associated with chiral fermions in Dirac or Weyl semimetals. The use of negative magnetoresistance (negative MR) as a signature for this anomaly remains contentious, as trivial mechanisms such as current jetting and weak localization can also induce negative MR. In this study, we report a novel nonlinear behavior of the chiral anomaly in the longitudinal direction, which we observed by applying parallel current and magnetic field to the Dirac semimetal Cd3As2. This nonlinear characteristic peaks at an intermediate magnetic field of approximately 5 T, displaying a resistance-increasing property concomitant with strengthening of the current source. Through angle-dependence experiments, we were able to rule out trivial factors, such as thermal effects, geometric artifacts, and anisotropy. Furthermore, additional electric quantum oscillations were observed when the direct current (DC) was applied as high as 300 μA. Such an unusual phenomenon is ascribed to the formation of quantized levels due to Bloch oscillation in the high DC regime, suggesting that an oscillatory density distribution may arise as the electric field increases. The non-Ohmic electric quantum oscillations open a new avenue for exploring chiral anomaly and other nontrivial topological properties, which is also one of the salient features of nonequilibrium steady states in condensed matter physics.

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