Abstract
A theoretical analysis of an adiabatic non-isothermal single-pellet diffusion reactor shows that non-isothermal effects can alter the value of the centerplane concentration. Deviation from isothermal behavior is significant under exothermic conditions where multiplicity of solutions can lead to reactor instabilities or falsification of reaction parameters. Conversely, it is shown that the internal isothermal model is a good approximation to detect non-isothermal pellet behavior from centerplane concentration measurements.
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