Abstract
In the flue emission from an internal combustion system using diffusing combustion such as coal or oil fuel boiler, incinerator, or diesel engine, around 10% oxygen is usually included. It is difficult to reduce the NO/sub x/ in the emission completely using catalysts or plasma alone because part of the NO/sub x/ is oxidized under an O/sub 2/-rich environment. In order to overcome these difficulties, we proposed a new after treatment system of NO/sub x/ included in the exhaust gas of the combustion system using nonthermal plasma (NTP) desorption and reduction. In this system, exchangeable adsorbent columns are equipped. First, the exhaust gas including NO/sub x/ is adsorbed to an NO/sub x/ adsorbent for a period of /spl Delta/t/sub a/. After the period of /spl Delta/t/sub a/, the path of the exhaust gas is changed with a pair of rotary valves and NO/sub x/ adsorbent is changed. The adsorbed NO/sub x/ is desorbed from the adsorbent and reduced by applying NTP for a period of /spl Delta/t/sub d/ using N/sub 2/ or low-oxygen-concentration gas. The exhaust gas is always kept clean by the exchange of adsorbent. Further, total electric energy can be reduced because NTP is not applied for /spl Delta/t/sub a/. This system can be operated at atmospheric temperature because no catalyst is used. As an initial step to realize such kind of after treatment system, the basic characteristics of the N/sub 2/ NTP desorption and NO/sub x/ reduction were examined experimentally using a pulse corona NTP reactor. After several adsorption/desorption processes, the amount of NO/sub x/ adsorbed becomes equal to that of the NO/sub x/ desorbed, that is, all the NO/sub x/ was desorbed in a single desorption process. It is confirmed that the NO/sub x/ complete reduction using N/sub 2/ NTP desorption is possible not only for a simulated exhaust gas but for a real diesel engine gas. The effective specific energy density can be decreased down to 22 Wh/m/sup 3/.
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