Abstract

NMR study of the organic conductor, (CH 3) 4P[Pd(dmise) 2] 2 has been performed. It was found that this compound exhibits a magnetic transition at 30 K. The transition temperature was higher than that of the isostructural sulfur analog, β-(CH 3) 4N[Pd(dmit) 2] 2 at ambient pressure (12 K). The electronic states in the insulating phases in this family are comparatively discussed on the basis of the 1H-NMR analyses.

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