Abstract
Considering the environment protection, “green” materials are increasingly explored for photovoltaics. Here, we developed a kind of quantum dots solar cell based on nitrogen-doped carbon dots. The nitrogen-doped carbon dots were prepared by direct pyrolysis of citric acid and ammonia. The nitrogen-doped carbon dots’ excitonic absorption depends on the N-doping content in the carbon dots. The N-doping can be readily modified by the mass ratio of reactants. The constructed “green” nitrogen-doped carbon dots solar cell achieves the best power conversion efficiency of 0.79 % under AM 1.5 G one full sun illumination, which is the highest efficiency for carbon dot-based solar cells.Electronic supplementary materialThe online version of this article (doi:10.1186/s11671-016-1231-1) contains supplementary material, which is available to authorized users.
Highlights
Among the third-generation photovoltaics, quantum dot solar cells (QDSCs) are emerging as a promising candidate due to the unique and versatile characteristics of quantum dots (QDs) including tunable band gap and high absorption coefficient [1–4]
Low-band gap metal chalcogenide (CdS, CdSe, CdTe, PbS, PbSe, CuInS2, etc.) QDs are widely used as sensitizers in QDSCs [5–10]
We have developed NCDs to build up the “green” QDSCs with enhanced efficiency
Summary
Among the third-generation photovoltaics, quantum dot solar cells (QDSCs) are emerging as a promising candidate due to the unique and versatile characteristics of quantum dots (QDs) including tunable band gap and high absorption coefficient [1–4]. Low-band gap metal chalcogenide (CdS, CdSe, CdTe, PbS, PbSe, CuInS2, etc.) QDs are widely used as sensitizers in QDSCs [5–10]. Mirtchev et al [24] have prepared water soluble CDs as sensitizers for QDSCs achieving power conversion efficiency (PCE) of 0.13 %. We have developed NCDs to build up the “green” QDSCs with enhanced efficiency. The NCDs with optimal excitonic absorption were used as sensitizers in the QDSCs. The constructed NCD solar cell achieves the best PCE of 0.79 % under AM 1.5 G one full sun illumination.
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