Abstract
We have demonstrated a novel approach to achieve a stable second-order NLO polymer by incorporating NLO moieties into a processable epoxy polymer and hardening with crosslinkable sol-gel technique. The crosslinked polymer showed high nonlinearity (d 33 = 41 pm/V) and better thermal stability compared to the prepolymer, which maintained its nonlinearity up to 100°C without significant loss of NLO activity.
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