Abstract
(C n H 2 n+1 NH 3) 2MnCl 4 consist of perovskite-type layers sandwiched between hydrocarbon radical layers. New phase transitions were found between liquid nitrogen and decomposition temperature in these compounds by differential thermal analysis and hot stage microscopy. A systematic research of the lattice dynamics, the transition mechanisms, their influence on physical properties and their dependence on the various possibilities of molecular engineering offered in these quasi two-dimensional perovskites was started.
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