Abstract
In the UV photolysis of perfluorinated alkyl iodides, iodine atoms in the two spin states 2P12 and 2P32 of the electronic ground state are formed. The atoms recombine in a three-body collision to form iodine molecules. The reactive collision of I(2P32) with I(2P12) leads to I2(B) which is detected by its chemiluminescence spectrum. The observed spectra contain an additional emission which is discussed to be the result of a transition from a higher excited I2 state correlating with two I(2P12).
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