New cold and ultra hot binary and cold ternary spontaneous fission modes for 252Cf and new band structures with gammasphere

Abstract

Prompt γ-γ-γ and x-γ-γ coincidence studies following the spontaneous fission of 252Cf were carried out first at Oak Ridge then at Gammasphere first with 36 and later with 72 Ge and two x-ray detectors and a long x-ray-γ coincidence experiment at Idaho. Many new cases of correlated pairs in cold (zero neutron emission) binary fission are observed and for the first time the heavier correlated pairs are identified in ternary fission where the third partners are α, 6He (or α2n), 10Be and, tentatively, 14C. Theoretical calculations were carried out of the relative yields of cold binary and ternary fission. There is reasonable agreement between the relative theoretical and experimental yields. New level structures and isotopes include new octupole deformations, identical bands and other structures. Stable octupole deformation is now observed in N=86, 140Xe, 142Ba and 144Ba and 143Ba, 148Ba and to higher spin in 144Ba. The 142–146Ba data provide the first evidence for the predicted disappearance of stable octupole deformation at high spins from band crossings. Identical yrast bands are observed with widely different neutron and proton numbers in 98,100Sr, 108,110Ru, 112,116Pd, 144,146Ba, 152,154,156Nd, 156Sm, 160Gd and a new type of shifted identical bands in 156,158,160Sm as well as the first identical octupole bands in 142,144Ba. Other new level structures are found. Yields and neutron multiplicities were measured directly for SrNd, ZrCe, MoBa, RuXe, and PdTe correlated pairs. A new ultra hot fission mode was discovered going via only 108Mo 144Ba, 107Mo 145Ba, and/or 106Mo 146Ba pairs where one or more of 44,145,146Ba are hyperdeformed at scission with 3:1 axis ratio.