Neutronic evaluation of the steady-state operation of a 20 kWth Aqueous Homogeneous Reactor for Mo-99 production

Abstract

Nowadays, 99mTc is the most common radioisotope used in nuclear medicine, with up to 30–40 million procedures worldwide every year. Furthermore, medical diagnostic imaging techniques using 99mTc represent approximately 80% of all nuclear medicine procedures. Currently, 99mTc is almost exclusively produced from the beta-decay of its 66-h parent 99Mo. The 99Mo production in an Aqueous Homogeneous Reactor (AHR) is potentially advantageous because of its low cost, small critical mass, inherent passive safety, and simplified fuel handling, processing, and purification characteristics. This paper studies an AHR conceptual design using low-enriched uranium for the production of 99Mo. Aspects related to the neutronic behavior such as critical height, medical isotopes production, uranium consumption, plutonium production and the reactivity feedback introduced in the solution by the volumetric expansion of the fuel solution were evaluated using the computational code MCNPX version 2.6e. In addition, important reactor kinetic parameters such as the effective delayed neutron fraction, βeff, and mean neutron generation time, Λ, were calculated. A benchmarking exercise was solved using available results of critical experiments performed at the Russian Research Center “Kurchatov Institute”. The neutronic calculations demonstrated that the reactor is able to produce 99 six-day Ci of 99Mo in operation cycles of five days. The reactivity feedbacks introduced by the volumetric expansion of the fuel solution is at about −1460 pcm, which represents approximately the 48% of the planned initial reactivity reserve in the core. The calculated effective delayed neutron fraction and the average mean neutron generation time were 785 pcm and 134.08 µs, respectively.