Abstract

An inverted-geometry white beam TOF neutron spectrometer using an extended graphite crystal analyzer was constructed at the CP-5 reactor at Argonne. A performance test of the spectrometer for incoherent inelastic scattering studies was made with five selected molecular solids. The results demonstrate the utility of such a spectrometer for investigation of lattice vibrational spectra of hydrogenous compounds in the energy range 0–400 cm−1. We describe design considerations and energy resolution of the spectrometer, and discuss observed low-frequency spectra of acetic acid (CH3COOH, CD3COOH, and CH3COOD), cyclohexane, and cyclopentane.

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