Abstract

Neutron Larmor Diffraction is a relatively new concept in neutron scattering which allows high resolution studies of subtle structural features in condensed matter. Several setups exist in various neutron facilities around the world. One of them is the Zero-field spin-Echo for Triple-Axis option (ZETA), available on the thermal triple-axis spectrometer IN22 (CEA-CRG beamline at Institut Laue Langevin). We have used ZETA to study thermal evolution of lattice constants in serveral systems of physical interest. Among them, the BaM2(XO4)2 family is a serie of compounds which have been intensively studied for three decades, mainly because of their fundamental though puzzling magnetic properties. In this paper, we aim to shed a new light on the physical understanding of those systems by investigating the link between structural and magnetic ordering. The magnetoelastic effect is found to be weak but can be resolved thanks to the high resolution provided by NLD.

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