Neutron calorimeter development at fission and fusion pulsed neutron sources

Abstract

A neutron calorimeter fielded in pulsed neutron irradiation experiments at the National Ignition Facility (NIF) and White Sands Missile Range Fast Burst Reactor (WSMR FBR) is described, and results are provided and discussed. The calorimeter is modular in design to allow fielding of various neutron absorber materials and thicknesses, as well as use at both fission and fusion sources, all of which has been done. Neutron calorimeters designed for fission sources have been fielded at fusion sources as well, but these instances are not documented in available literature—making this work novel. The functional calorimeter consists of a neutron absorber and two sheathed, grounded thermocouples secured within a subassembly made of thermally insulating materials. This subassembly is placed into a sealed vessel for material and facility safety considerations. The device was fielded at NIF in four polar-direct-drive exploding pusher shots and eleven WSMR FBR pulses. Calorimeter data from NIF experiments show a discernable thermal response accredited to neutron heating within the first 10 s, but the data are dominated by noise from ambient X-ray heating after time = 10 s post-pulse. This response is highly consistent between shots and linearly related to incident neutron fluence and neutron absorber thickness. A temperature rise of 1.1E−2 K/(1013 neutrons/cm2) per millimeter of absorber thickness was determined for both 0.4 mm and 1 mm thick depleted uranium absorbers with linear best fit R2 of 0.97 and 0.98 for each thickness and y-axis offsets of 8.8E−3 and 1.3E−2, respectively. WSMR FBR experiment data show a temperature rise of 6.2E−2 K/(1013 neutrons/cm2) with linear best fit R2 of 0.14 and y-axis offset of 7.6E−3 for a calorimeter with a 1 mm thick enriched boron carbide (10B4C) absorber, though it must be noted that device-to-device variability is significant at both facilities. These data are also affected by noise on a similar timescale as at NIF, though the noise is significantly lesser in magnitude but oscillatory.