Abstract

Trustworthy technology for the monitoring of fugitive methane emissions is an indispensable component for low−carbon emission reduction and safe production in oil and gas infrastructure. A miniaturization and low-cost methane remote monitoring prototype based on near-infrared laser absorption spectroscopy is developed to retrieve the path−integral concentration by employing the harmonic conjoint analysis method for the backscattered echo signals from a distant non-cooperative target. A distorted harmonic template matching (DHTM) algorithm is proposed based on wavelength modulation spectroscopy with second harmonic normalized via the first harmonic (WMS−2f/1f) method, which suppresses the output concentration fluctuation caused by open path monitoring with non-cooperative target and avoids the issue of false alarms during the detection process without target gas. The reliability of the WMS−2f/1f−DHTM algorithm is verified by calibration and dynamic experiments. The results showed that this algorithm avoids the dilemma of false alarms in the absence of gas compared to the conventional WMS−2f/1f algorithm, while the root mean square error (RMSE) of the concentration inversion with a detection distance of 20 m is reduced by 57.6% compared to direct absorption spectroscopy (DAS) algorithm. And the minimum detection limit of system is 3.79 ppm·m. The methane telemetry sensor with the WMS−2f/1f−DHTM algorithm exhibits substantial application potential in carbon monitoring of oil and gas industry.

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