Abstract
Chemical deposition is used to obtain thin solid films of lead sulfide Pb(S, O) with oxygen contents of 0.2 to 30.7 at %, regulated by a variety of ligands. The oxygen effect on the mechanism of formation and optical properties of Pb(S, O) films is studied experimentally and through quantum-chemical modeling. A heterostructured nature of the synthesized Pb(S, O) compounds is shown for the first time, and a mechanism of their formation in an aqueous solution is proposed.
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