Abstract

Two-dimensional atomic heterostructures combined with metallic nanostructures allow one to realize strong light–matter interactions. Metallic nanostructures possess plasmonic resonances that can be modulated by graphene gating. In particular, spectrally narrow plasmon resonances potentially allow for very high graphene-enabled modulation depth. However, the modulation depths achieved with this approach have so far been low and the modulation wavelength range limited. Here we demonstrate a device in which a graphene/hexagonal boron nitride heterostructure is suspended over a gold nanostripe array. A gate voltage across these devices alters the location of the two-dimensional crystals, creating strong optical modulation of its reflection spectra at multiple wavelengths: in ultraviolet Fabry–Perot resonances, in visible and near-infrared diffraction-coupled plasmonic resonances and in the mid-infrared range of hexagonal boron nitride's upper Reststrahlen band. Devices can be extremely subwavelength in thickness and exhibit compact and truly broadband modulation of optical signals using heterostructures of two-dimensional materials.

Highlights

  • Two-dimensional atomic heterostructures combined with metallic nanostructures allow one to realize strong light–matter interactions

  • The gold plasmonic nanostripe array is separated from the graphene/hexagonal boron nitride (hBN) by an air gap (d)

  • Our modulator design could be adapted to detect the motion of a 2D heterostructure by measuring the dispersive coupling strength g 1⁄4 DE/Dz, where DE is the shift in the collective plasmon energy and Dz the displacement of the membrane

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Summary

Introduction

Two-dimensional atomic heterostructures combined with metallic nanostructures allow one to realize strong light–matter interactions. The advent of high-resolution nanofabrication techniques has allowed for the development of plasmonic nanostructures with a broad range of optical responses such as subwavelength confinement of light[4] and ultra-narrow diffraction-coupled resonances[5,6,7] that could lead to applications in waveguiding[8] and biosensing[9], respectively. Combining graphene with metallic nanostructures capable of supporting ultra-narrow plasmon resonances could potentially lead to the development of compact optical modulators[3]. Application of a gate voltage between graphene and the gold nanostripe sublayer leads to a reduction in the air gap height This in turn changes the effective electric field acting on graphene and hBN, modifying spectral reflection features from mid-ultraviolet to mid-infrared wavelengths. In the mid-infrared region (at a wavelength l B7 mm) the optical interrogation volume is Bl3/10, the smallest reported so far—approximately three orders of magnitude smaller than reported in ref

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