Abstract

In article number 1803471, Johnas Eklöf-Österberg, Kasper Moth-Poulsen, and co-workers make isolation, positioning, and electronic measurements on single molecules possible using a combined top-down and bottom-up strategy. Proto-devices, which are self-assembled nanogaps composed of two gold nanoparticles linked by a single or a few molecules, are guided onto top-down prefabricated nanosized electrodes by surface charge interactions. The assembly process enables electrical measurements through particle–molecule–particle devices.

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