Abstract

Li-Ion Battery Cathodes In article 2208423, Hyun-Wook Lee, Jinhyuk Lee, Dong-Hwa Seo, and co-workers reveal the multiphase heterogeneous nature of ultrahigh-energy Mn-based partially disordered Li-ion cathodes through combined experimental and computational studies. This fundamental understanding enables novel nanocomposite design, wherein a phase fraction of the nanocomposites is manipulated. Consequently, cathodes engineered via nanocomposite engineering exhibit superior reversible redox properties and improved cycle retention.

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