Abstract
The statistical properties of fluorescence photon emission of single molecule modeled by two-level system (TLS) under pump-probe fields were investigated by employing the generating function method developed recently. We study the impact of pump-probe fields on some single molecule statistical properties, such as, the line shapes, Mandel Q parameters and probalities of photon emission. Our theoretical result about average emission photon numbers and experimental result are in good agreement.
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More From: SCIENTIA SINICA Physica, Mechanica & Astronomica
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