Abstract
Local-probe weak-transverse-field and zero-field μSR measurements have been employed to investigate magnetic ordering in the new magnetoelectric compound FeTe2O5Br. Below the Néel transition temperature TN=10.6 K a static local magnetic field starts to develop at the μ+ sites. Fast μ+ polarization decay below TN speaks in favor of a broad distribution of internal magnetic fields, in agreement with the incommensurate magnetic structure suggested by neutron diffraction experiments. Above TN the presence of short-range order is detected as high as at 2TN, which suggests only weak interlayer magnetic coupling. On the other hand, strong Fe3+ spin fluctuations likely reflect geometrically frustrated structure of [Fe4O16]20− spin clusters, which are the main building blocks of the layered FeTe2O5Br structure.
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