Abstract

In this paper we overview our work on far-infrared spectroscopy of both hetero- and homonuclear diatomic molecules in nonpolar fluids. Special attention is paid to electric multipolar induced contributions. From comparison between theoretical and experimental spectra estimation of the leading multipoles of CO and N2 molecules has been obtained. Also a temperature and density dependence analysis of many-body cancellation effects in the different pure induced components of the far-infrared integrated absorption coefficient of CO in liquid Ar is reported.KeywordsDipole MomentDiatomic MoleculeRotational ComponentMultipole MomentPermanent Dipole MomentThese keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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