Abstract

The femtosecond-laser-writing technique provides a flexible method for fabrication of nonlinear photonic crystals in three dimensions, providing structures that enable efficient complex nonlinear wave interactions and modulation for applications including nonlinear holography, nonlinear beam shaping, and waveguide-integrated wavelength conversion. However, the tightly focused laser pulse inevitably causes structural modification and then changes the local refractive index, resulting in additional linear modulation of the interacting waves. Here, we use the same periodic distributions of the refractive index and the second-order nonlinear coefficient for grating arrays engineered in lithium niobate crystals by femtosecond laser writing to achieve polarization-dependent linear and nonlinear Bragg diffractions simultaneously. The experimental results show that the linear and nonlinear diffraction efficiencies range up to 31% and 2.9 × 10−5, respectively, for grating arrays with dimensions of 100 μm (x) × 100 μm (y) × 100 μm (z). This work paves the way toward the realization of the multiplexing of linear and nonlinear optical modulations in a single structure for potential applications that include multidimensional optical data storage and optical coding.

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