Multiplex vortex instability in the flow of non-Newtonian fluids through microcavity arrays

Abstract

Complex fluids always possess obvious non-Newtonian properties that facilitate the occurrence and development of vortex instability in porous media, which is of critical significance in many natural and industrial processes. It is widely known that this flow instability is regulated by both fluid flow and solid structure. However, the quantitative understanding of how structural characteristics of porous space affect the evolution of vortex instability is still nascent, especially in the case of fluids with varying rheological properties. Herein, the flow of polymer solutions with distinct non-Newtonian properties through microcavity arrays is experimentally studied, by which we systematically explore the effect of structural parameters of the cavity array on vortex instability. We find that, for both Newtonian and shear-thinning fluids with negligible elasticity, the vortex evolution behavior in each cavity of the cavity array is identical to those in an isolated cavity. In contrast, for viscoelastic fluids, the vortex instability is visibly affected by cavity number and cavity–cavity interval, and this effect exhibits different forms when the fluid shear-thinning participates or not. Multiplex vortex instabilities are observed under these tested conditions. By multiplex, we mean the vortex formation dynamics and evolution patterns are diversified. These unusual evolution phenomena are then interpreted in terms of the interplay between the elongation and relaxation of polymers as they navigate among neighboring cavities. These results can help us to further understand the flow instability of complex fluids in porous media and evoke new strategies for microfluidic applications of efficient mixing.