Abstract

N( 2D) has been detected by resonance-enhanced multiphoton ionization (REMPI) at 269 nm in both the products of a microwave discharge in nitrogen (0.2–2%) in argon mixtures and as a result of two-photon dissociation of N 2O. Further increase in the nitrogen fraction through the discharge decreased the N( 2D) signal and finally replaced it with a series of molecular bands whose origin is thought to be electronically excited metastable states of N 2.

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