Abstract

We present the results of multiobjective genetic algorithm optimizations of a single-shot ultrafast electron diffraction beam line utilizing a 225 kV dc gun with a novel cryocooled photocathode system and buncher cavity. Optimizations of the transverse projected emittance as a function of bunch charge are presented and discussed in terms of the scaling laws derived in the charge saturation limit. Additionally, optimization of the transverse coherence length as a function of final rms bunch length at the sample location have been performed for three different sample radii: 50, 100, and $200\text{ }\text{ }\ensuremath{\mu}\mathrm{m}$, for two final bunch charges: $1{0}^{5}$ electrons (16 fC) and $1{0}^{6}$ electrons (160 fC). Example optimal solutions are analyzed, and the effects of disordered induced heating estimated. In particular, a relative coherence length of ${L}_{c,x}/{\ensuremath{\sigma}}_{x}=0.27\text{ }\text{ }\mathrm{nm}/\ensuremath{\mu}\mathrm{m}$ was obtained for a final bunch charge of $1{0}^{5}$ electrons and final bunch length of ${\ensuremath{\sigma}}_{t}\ensuremath{\approx}100\text{ }\text{ }\mathrm{fs}$. For a final charge of $1{0}^{6}$ electrons the cryogun produces ${L}_{c,x}/{\ensuremath{\sigma}}_{x}\ensuremath{\approx}0.1\text{ }\mathrm{nm}/\ensuremath{\mu}\mathrm{m}$ for ${\ensuremath{\sigma}}_{t}\ensuremath{\approx}100--200\text{ }\text{ }\mathrm{fs}$ and ${\ensuremath{\sigma}}_{x}\ensuremath{\ge}50\text{ }\text{ }\ensuremath{\mu}\mathrm{m}$. These results demonstrate the viability of using genetic algorithms in the design and operation of ultrafast electron diffraction beam lines.

Highlights

  • Electron diffraction [1] has become a valuable measurement technique with modern ultrafast electron diffraction (UED) experiments [2,3,4,5,6,7,8,9] capable of atomic level observation of structural dynamics using single-shot tabletop sized setups [4,7]

  • The beam line is comprised of a 225 kV dc gun featuring a cryocooled photocathode, a separate bunching cavity, and two solenoid magnets

  • The design of the dc gun, in particular the operating voltage (225 kV) and cathode gap (20 mm), represents a realistically feasible solution based on empirical high voltage break down limits

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Summary

INTRODUCTION

Electron diffraction [1] has become a valuable measurement technique with modern ultrafast electron diffraction (UED) experiments [2,3,4,5,6,7,8,9] capable of atomic level observation of structural dynamics using single-shot tabletop sized setups [4,7]. Advances in the development of low mean transverse energy (MTE) photocathodes [17,18], as well as both dc gun and normal conducting rf (NCRF) gun technology [19,20], promise to provide electron beams with ever increasing brightness (low emittance). Application of this technology in UED beam lines opens up the possibility for atomic resolution of increasingly complicated systems with larger unit cells. Examples for σx ≈ 50 μm are simulated for both final charges, and the dynamics in each case discussed

Coherence length from photocathode sources
ONE APPROACH FOR OPTIMAL COHERENCE LENGTH
RESULTS
Optimal emittance
Optimal coherence length
CONCLUSIONS
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