Abstract
HighlightsThe interfacing between SnO2 and MXene alters electronic structures, shifting the d-band center in transition metals, enhancing catalytic efficiency by reducing electron filling in antibonding orbitals.A binder-free, ultrathin, laminar heterostructured interlayer on polypropylene separator is demonstrated. The ionic sieving mechanism and efficient adsorption–catalysis process enable deeper charge/discharge cycle and improved stability.The improved catalytic conversion and suppressed lithium dendrites formation enable a high loading of 7.5 mg cm−2 and an initial area capacity of 7.6 mAh cm−2.
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