Abstract

The polarization of high-order harmonic radiation emitted from ${\mathrm{N}}_{2}$ molecules interacting with a linearly polarized laser pulse is investigated theoretically. We find that the exchange effect between the recombining electron and the bound core electrons imprints a clear signature onto the high-order harmonic polarization and its dependence on the alignment angle between the molecular axis and driving laser electric field. Our analysis reveals an observable for the experimental investigation of many-electron dynamics in intense laser fields.

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